Abstract
The basic rules of the approach to study of the mechanism of photobreak of chemical bonds in complex molecules of linear and cyclic structure by methods of quantum chemistry are stated. Photolysis of disulfides, chlornaphthalenes, diphenyloxazones, thrinitrotoluene, coumarine is investigated by offered method. Mechanisms of primary photoreactions are revealed. Electronic excited states are established, in which there is the break of chemical bond, and opportunity them occupation.
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