Abstract

We explored a Mg-alloyed ZnO material (or MgZnO alloy) on a lattice-matched scandium aluminum magnesium oxide substrate for obtaining most effective photodetectors with highest (∼10 A/W) and fastest (up to 3 GHz) responses and two orders of magnitude UV/VIS rejection ratio. Device operation was related to its material electronic properties (carrier lifetime, diffusivity, and diffusion length) via photoluminescence and light-induced pump–probe techniques. Defect-related response is found suitable for sensitive logarithmic detectors, while exciton-related response is favorable to ultrafast linear UV solar blind detectors. Two-contact planar detector design allows their application in low-cost environmental detection systems.

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