Kinetics of Stimulated Polariton Scattering in Planar Microcavities: Evidence for a Dynamically Self-Organized Optical Parametric Oscillator

Abstract

Strong temporal hysteresis effects in the population kinetics of pumped and scattered lower polaritons (LPs) have been observed in a planar semiconductor microcavity under a nanosecond-long pulsed resonant excitation (by frequency and angle) near the inflection point of the LPs' dispersion. The hysteresis loops have a complicated shape due to the interplay of two instabilities. The self-instability (bistability) of the nonlinear pumped LP is accompanied by a strong parametric instability which causes an explosive growth of the scattered LPs' population over a wide range of wave vectors. Finally, after a 30-500 ps period, a three-mode scattering pattern forms, thereby demonstrating a dynamically self-organized regime of the optical parametric oscillator. Stability is maintained by the presence of numerous weak "above-condensate" modes; the whole system therefore appears to be highly correlated.