Abstract
AbstractThe [3+2] annulation of N‐sulfonyl aromatic imines with 1,3‐dienes proceeded via a direct CH functionalization to give 1‐aminoindane derivatives in high yields with high regio‐ and stereoselectivities. The iridium complex coordinated with a substrate 1,3‐diene displayed high catalytic activity. The reaction proceeds via the direct formation of the aryliridium(I) species from the aromatic aldimine and an iridium(I) acetate species via a concerted metalation‐deprotonation pathway.magnified image
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