Abstract
In this talk, I will highlight some of our recent advances in the field of direct electrochemical reduction of CO2 into value-added fuels and chemicals on non-metallic carbon-based MNC electrocatalysts with molecularly-defined coordinative MNx metal-nitrogen centers as active sites. Special focus will be placed on efficient production of CO at lab-scale and industrial current densities with emphasis on a fundamental understanding of between selectivity and the nature of the MNx moiety. Furthermore, the design of hybrid electrocatalysts consisting of CO-efficient MNC backbones decorated with CuOx nanoparticles will be addressed and the molecular mechanisms of their enhanced ethylene production discussed.
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