Abstract
Colloidal nanoparticles with anisotropic interactions are promising building blocks for the fabrication of complex functional materials. A challenge in the self-assembly of colloidal particles is the rational design of geometry and chemistry to program the formation of a desired target structure. We report an inverse design procedure integrating Langevin dynamics simulations and evolutionary algorithms to engineer anisotropic patchy colloidal clusters to spontaneously assemble into a cubic diamond lattice possessing a complete photonic band gap. The combination of a tetrahedral cluster geometry and optimized placement of a single type of anisotropic interaction patch results in a colloidal building block predicted to assemble a cubic diamond lattice with more than 82% yield. This design represents an experimentally viable colloidal building block capable of high-fidelity assembly of a cubic diamond lattice.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
