Abstract

Long-lived circular Rydberg atoms are picking up increasing interest for boosting coherence times in Rydberg-based quantum simulation. We elaborate a novel approach to stabilize circular Rydberg states against spontaneous and blackbody-induced decay using a suppression capacitor made from indium tin oxide (ITO) thin films, which combine reflection of microwaves with transparency in the visible spectral range. To this end, we perform detailed characterization of such films using complementary spectroscopic methods at GHz and THz frequencies and identify conditions that allow for reaching circular-state lifetimes up to tens of milliseconds in a room-temperature environment. We discuss prospects of our findings in view of the quest for quantum simulations with high-$n$ circular Rydberg states at room temperature.

Highlights

  • Ultracold Rydberg atoms have recently shown fascinating means for realizing a versatile platform for applications in quantum simulation and quantum information processing

  • We report on detailed millimeter-wave investigations of indium tin oxide (ITO) thin films of different thickness and sheet resistance using a combination of complementary spectroscopy methods, which allow us to infer microwave properties of the films covering a frequency range from 100 MHz up to 1 THz

  • We have elaborated a new approach to stabilize high-n circular Rydberg states against spontaneous and blackbody-induced decay in a transparent, microwave-reflecting cavity formed by ITO-coated glass plates

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Summary

INTRODUCTION

Ultracold Rydberg atoms have recently shown fascinating means for realizing a versatile platform for applications in quantum simulation and quantum information processing. Circular Rydberg atoms have been extensively explored in atomic beam experiments [10,11,12] Their individual interaction with microwave photons trapped in high-quality resonators allowed for fundamental studies of cavity quantum electrodynamics [13]. A quantum simulator based on very long-lived circular Rydberg states should allow for optical trapping inside a microwave resonator, which poses stringent limitations for optical access and for trapping ensembles of atoms in defect-free tweezer arrays [9]. We explore the feasibility to realize a capacitor for suppressing high-n circular Rydberg state decay with indium tin oxide (ITO) films [Fig. 1(a)] Such a capacitor has to combine high reflectivity in the microwave domain with transparency for visible to short near-infrared wavelengths. To stabilize circular Rydberg states for tens of milliseconds even in a room temperature environment

Radiative decay of circular Rydberg states
Stabilizing circular Rydberg states in a cavity
ITO THIN FILMS AT GHz AND THz FREQUENCIES
Experimental methods
GHz and THz characteristics of ITO thin films
THz reflection and transmission
Optical conductivity
PROSPECTS FOR A CIRCULAR RYDBERG ATOM
CONCLUSION AND OUTLOOK
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