Abstract

We perform in-plane optical spectroscopy measurement on (00l) FeSe thin film grown on SrTiO${}_{3}$ substrate by the pulsed laser deposition method. The study indicates that the low-frequency conductivity consists of two Drude components: a broad one which takes up most of the spectral weight and a very narrow one roughly below 100--150 cm${}^{\ensuremath{-}1}$. The narrow Drude component locates at so low frequencies that no such behavior was observed in iron pnictides. The overall plasma frequency is smaller than that of the FeAs-based compounds, suggesting a stronger correlation effect. Similar to iron pnictides, a temperature-induced spectral weight transfer is observed for FeSe. However, the relevant energy scale is smaller. Additionally, different from a recent angle-resolved photoemission spectroscopy measurement which revealed a spin density wave (SDW) order at low temperature for FeSe thin films grown on SrTiO${}_{3}$ substrate, no signature of the band structure reconstruction arising from the formation of the SDW order is seen by optical measurement in the thick FeSe films.

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