Abstract
Electron and Ion transport systems often rely on a balanced hierarchical boundary structure that spans from millimetre to nanometer scales. Systematically varied polymers and organic crystals are used to fine-tune the growth of soft nanostructured complexes. (1-2) The underlying intermolecular interactions between crystallization mediator and small molecule crystals can lead to thin films of largely enhanced performance for charge transport and energy storage purposes. In this work, controlled solution deposition was used to self-assemble a number of novel organic capacitors and solid electrolyte systems based on semicrystalline polymers, whose capacitance and ion conductivity are examined as a function of the resultant nanostructures and regulated crystallization conditions. Electrochemical impedance measurements, equivalent circuit modelling, as well as Vogel-Tamman-Fulcher relations are performed in light of microscopy studies including low-dose TEM to provide insights on capacitance enhancement and ion transport mechanism.(3)
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