Abstract

An approach for fabrication of planar devices integrating layered Bi2Te3 thin-films with different microscale thicknesses instead of bulk materials is reported. The films were prepared by the radio-frequency magnetron sputtering. The microstructure, composition, and thermoelectric (TE) properties of the thin-films were characterized using X-ray diffraction, scanning electron microscopy with energy dispersive X-ray spectroscopy, and a TE measurement system, respectively. The results show that the Bi2Te3 films with layered microstructure possess promising TE properties. The power generation and cooling performance of parallel micro-devices with n-type thermolegs were tested and found to be superior to those of bulk material devices. For a typical parallel device with 38 optimized 2-μm-thick legs, the output voltage, estimated maximum power and corresponding power density are up to 5.6mV, 6.53μW and 43mWcm−2, respectively, for a temperature difference of 81K. The coefficient of performance (COPmax) of the device was also estimated. The minimum value of COPmax approaches 6.8 at ΔT=3.2K. The results prove that high performance of micro-device with low internal resistance can be realized by integrating special layered Bi2Te3 thin-films.

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