Abstract
Oxidative conversion of methane, ethane, propane, benzene, hydrogen and their binary mixtures R1–R2–N 2O–He (where R1, R2 are substances under study) were studied on HZSM-5 at 350–450°C. Relative reactivities were estimated, rate of conversion of hydrocarbons correlating with the strength of CH bond. 13C label distribution in the product of 13CH 4–C 6H 6–N 2O feed was studied by GC-MS, 1H and 13C NMR. It was shown that methane was capable to alkylate the aromatic ring under reaction condition, giving toluene and xylenes from benzene.
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