Abstract

The rapid development of neuro-inspired computing demands synaptic devices with ultrafast speed, low power consumption, and multiple non-volatile states, among other features. Here, a high-performance synaptic device is designed and established based on a Ag/PbZr0.52Ti0.48O3 (PZT, (111)-oriented)/Nb:SrTiO3 ferroelectric tunnel junction (FTJ). The advantages of (111)-oriented PZT (~1.2 nm) include its multiple ferroelectric switching dynamics, ultrafine ferroelectric domains, and small coercive voltage. The FTJ shows high-precision (256 states, 8 bits), reproducible (cycle-to-cycle variation, ~2.06%), linear (nonlinearity <1) and symmetric weight updates, with a good endurance of >109 cycles and an ultralow write energy consumption. In particular, manipulations among 150 states are realized under subnanosecond (~630 ps) pulse voltages ≤5 V, and the fastest resistance switching at 300 ps for the FTJs is achieved by voltages <13 V. Based on the experimental performance, the convolutional neural network simulation achieves a high online learning accuracy of ~94.7% for recognizing fashion product images, close to the calculated result of ~95.6% by floating-point-based convolutional neural network software. Interestingly, the FTJ-based neural network is very robust to input image noise, showing potential for practical applications. This work represents an important improvement in FTJs towards building neuro-inspired computing systems.

Highlights

  • The rapid development of neuro-inspired computing demands synaptic devices with ultrafast speed, low power consumption, and multiple non-volatile states, among other features

  • The basic tasks of recognizing handwritten digits in the Modified National Institute of Standards and Technology (MNIST) database and more complicated fashion product images in the Fashion-MNIST (F-MNIST) database have been widely used to test the capability of neural network computing systems[17,18]

  • Pt/BaTiO3 (001)/Nb:SrTiO3 (NSTO)based ferroelectric tunnel junction (FTJ) with 200 states in a conductance dynamic range of 10× have been reported with an operation speed of 50 ns and an endurance of >1.1 × 104 cycles[24]

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Summary

Introduction

The rapid development of neuro-inspired computing demands synaptic devices with ultrafast speed, low power consumption, and multiple non-volatile states, among other features. A high-performance synaptic device is designed and established based on a Ag/ PbZr0.52Ti0.48O3 (PZT, (111)-oriented)/Nb:SrTiO3 ferroelectric tunnel junction (FTJ). It is commonly believed that to realize an efficient neuro-inspired computing system, it is necessary to develop high-performance synaptic devices that are based on memristors and capable of emulating the weight updates of biological synapses[4,5]. As a recently developed memristor strategy, the ferroelectric tunnel junction (FTJ) is in principle a promising candidate for building high-performance artificial synapses. This is because the FTJ stores data non-volatilely and intrinsically as ferroelectric polarization states in its ultrathin ferroelectric barrier. Based on the principle of the FTJ, multiple conductance states are related to multiple ferroelectric domains

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