Abstract
A novel high-conductivity Agx[(Ga2Te3)34(SnTe)66]100-x tellurium-based glassy system was fabricated via melt spinning with the glass formation area in the range of x = 0-15 mol %. A bulk Ag10[(Ga2Te3)34(SnTe)66]90 glass (A10) was obtained via spark plasma sintering at 450 K using a 5 min dwell time and 400 MPa pressure. The fabricated A10 glass exhibited higher room-temperature conductivity (σ300 K = 46 S m-1), larger glass transition temperature (Tg = 482 K), and ultralower thermal conductivity (∼0.19 W m-1 K-1) compared to those of previously reported Cu-Ge-Te, Cu-As-Te, Cu-Ge-As-Te, and Cu-As-Se-Te glassy systems with the approximate doping concentrations of 5-20%, demonstrating that this distinctive Ag-Ga2Te3-SnTe system is interesting materials for thermoelectric applications. The high-conductivity Ag-Ga2Te3-SnTe glassy system will extend investigations into similar glassy semiconductors and also can be used for preparing glass ceramics with potential applications in other fields.
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