Abstract

The generation of two independently tunable light pulses in the mid-infrared spectral region is reported here. Synchronously pumping two optical parametric oscillators in parallel with a flashlamp-pumped, pulsed Nd:YLF laser delivers tunable radiation in the range 1.2-1.7 /spl mu/m with duration of 300 fs. Subsequent parametric amplification in AgGaS/sub 2/ crystals yields intensive light pulses in the wavelength range of 2.7-7 /spl mu/m with duration of approximately 1 ps and energies up to 10 /spl mu/J. Pulse analysis determining also the zero delay time and the temporal resolution of the experimental system is performed via two-photon absorption in germanium, utilizing the direct band gap. The temporal resolution of the two-color IR-system is determined to be approximately 300 fs and first application to time-resolved spectroscopy in the condensed phase is demonstrated.

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