Abstract
A facile strategy is developed to fabricate 3nm RuIrOx nanocrystals anchored onto N-doped hollow carbon for highly efficient and pH-universal overall water splitting and alkaline seawater electrolysis. The designed catalyst exhibits much lower overpotential and superior stability than most previously reported Ru- and Ir-based electrocatalysts for hydrogen/oxygen evolution reactions. It also manifests excellent overall water splitting activities and maintains ≈100% Faradic efficiency with a cell voltage of 1.53, 1.51, and 1.54V at 10mAcm-2 for 140, 255, and 200h in acid, alkaline, and alkaline seawater electrolytes, respectively. The excellent electrocatalytic performance can be attributed to solid bonding between RuIrOx and the hollow carbon skeleton, and effective electronic coupling between Ru and Ir, thus inducing its remarkable electrocatalytic activities and long-lasting stability.
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