Abstract

Unambiguous experimental evidence for a significant difference in efficiency of excitonic vs. free carrier spin injection is provided in novel laterally arranged self-assembled InAs/GaAs quantum dot structures, from optical orientation and tunable laser spectroscopy. A lower efficiency of exciton spin injection as compared to free carrier spin injection from wetting layers into QDs results in a distinct feature in luminescence polarization of the QDs as a function of excitation photon energy. It is shown that this difference is not related to carrier density and state-filling effects arising from the difference in optical absorption efficiency between the excitons and free carriers. Rather, it is a genuine property for exciton spin injection that suffers stronger spin relaxation due to Coulomb exchange interaction.

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