Abstract

The Doppler-free two-photon spectra of the 6 S 1/2 ( F = 3)–6 D 3/2 ( F = 2 to 5), 6 S 1/2 ( F = 4)–6 D 3/2 ( F = 2 to 5), 6 S 1/2 ( F = 3)–6 D 5/2 ( F = 5 to 1) and 6 S 1/2 ( F = 4)–6 D 5/2 ( F = 6 to 2) transitions in cesium are observed using a titanium-sapphire laser. These spectra can be used as an optical frequency standard. The hyperfine coupling constants A (magnetic dipole constant) and B (electric quadrupole constant) are determined using spectral line splittings, giving A = 16.17(17) MHz and B = 0.11(127) MHz for the 6 D 3/2 state, and A =-4.56(9) MHz and B = -0.35(183) MHz for the 6 D 5/2 state.

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