Abstract
Electron paramagnetic resonance studies performed at room temperature in Mn2+ doped Cs2NaLaCl6 single crystals (elpasolite type) showed that the Mn2+ ion occupies two different tetragonal symmetry sites in a cubic crystalline lattice. Both sites possess principal Z-axes along 〈100〉 crystallographic directions with large splittings (≊1.0 cm−1 and ≊0.8 cm−1) of the spectra. Several facts are taken into account in order to establish tentative models for the structural configuration of the two sites.
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