Abstract

Carbon nanotubes (CNTs) used as semiconducting channels induce high mobility, thermal conductivity, mechanical flexibility, and chemical stability in field-effect, thin-film transistors (TFTs). However, the contact interfaces in CNT-TFTs have contact resistances that are difficult to reduce; this contact resistance can eventually limit the overall performance of CNT-TFTs. The contact interface between the source/drain electrodes and CNTs, especially for those CNT-TFTs in which the channel comprises randomly networked CNTs, plays a particularly dominant role in determining the performance and degree of variability in CNT-TFTs. However, no studies have reported a determination method that individually extracts each contact resistance at the source/drain electrodes. The present work presents an efficient method for directly determining the contact interfaces in CNT-TFTs by extracting each contact resistance produced at the source (RS) and drain (RD) electrodes. Moreover, we comprehensively simulated the randomly networked CNTs using an in-depth Monte-Carlo method, which provides an efficient method for visualizing the uniformity of a CNT network with various controllable CNT parameters. The proposed method provides guidance and a means for optimizing the design of the CNT network channel in CNT-TFTs and additional insights into improving the performance of CNT-TFTs.

Highlights

  • Carbon nanotubes (CNTs) have been intensely studied for use as channel materials in thin-film transistors (TFTs) due to their high carrier mobility, excellent chemical stability, mechanical flexibility, and compatibility with solution-based processing[1,2,3,4,5,6,7,8,9,10,11]

  • The fabrication of CNT-TFTs started from the silicon wafer, which was highly p-doped to serve as the global back-gate, with a thermally grown 55-nm-thick silicon dioxide (SiO2) layer

  • The CNT network channel was formed by immersing the chip into a 99% semiconducting enriched CNT solution (0.01 mg/ ml) for three different times of 6, 8, and 10 h, followed by thorough rinsing with isopropanol and DI water

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Summary

Introduction

Carbon nanotubes (CNTs) have been intensely studied for use as channel materials in thin-film transistors (TFTs) due to their high carrier mobility, excellent chemical stability, mechanical flexibility, and compatibility with solution-based processing[1,2,3,4,5,6,7,8,9,10,11].

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