Abstract
Herein, we created defects on NH2-MIL-125 to form more nodes of grafted metals, and synthesized a series of hybrid materials (Cu/d-NH2-MIL-125 and CuNPs/d-NH2-MIL-125 with 1,2, and 4 wt % of Cu nanoparticles) that were used as photocatalysts of the hydrogen evolution reaction and dehydrogenation of tetrahydroisoquinoline. At the optimal relative amount of Cu, namely 2 wt %, the hydrogen evolution reaction and dehydrogenation of tetrahydroisoquinoline showed rates of 1326.55 μmol g-1 h-1 and 427.15 μmol g-1 h-1, respectively. This new photocatalyst could effectively improve the e-/h+ separation efficiency, enriching the investigation of MOFs in the field of photocatalytic hydrogen evolution.
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