Abstract
The rational design of a chemically tunable reaction system to synthesize polyoxometalate (POM)-directed entangled metal–organic coordination networks is still a challenging but fascinating task. In their Full Paper on page 819 ff., Yong-Hui Wang, Fu-Chen Liu, and Yang-Guang Li et al. report a new reaction system containing charge-tunable Keggin-type POM units and the preparation of four new POM-directed entangled networks based on transition-metal (TM) ions and the ligand 1,4-bis(1,2,4-triazol-1-ylmethyl)benzene. In these compounds, the chemically charge-tunable Keggin-type POMs play a key role in changing the structural topologies of entangled networks and modulating the photocatalytic activities of hybrid compounds.
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