Science | VOL. 369
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Cooperative carbon capture and steam regeneration with tetraamine-appended metal–organic frameworks

Publication Date Jul 24, 2020

Abstract

Natural gas has become the dominant source of electricity in the United States, and technologies capable of efficiently removing carbon dioxide (CO2) from the flue emissions of natural gas–fired power plants could reduce their carbon intensity. However, given the low partial pressure of CO2 in the flue stream, separation of CO2 is particularly challenging. Taking inspiration from the crystal structures of diamine-appended metal–organic frameworks exhibiting two-step cooperative CO2 adsorption, we report a family of robust tetraamine-functionalized frameworks that retain cooperativity, leading to the potential for exceptional efficiency in capturing CO2 under the extreme ...

Concepts

Low Partial Pressure Of CO2 Flue Stream Steam Regeneration Low-temperature Steam Natural Gas Temperature Swings Carbon Intensity Simulated Flue Gas Pressure Swings Humid Gas

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