Abstract
Constructing an S-scheme system with highly active catalysts is a significant approach for improving the separation of photoinduced carriers to solve the related environmental aggravation. In this study, a well-designed S-scheme AgVO3/CaIn2S4 photocatalyst was synthesized for water purification by in situ growing CaIn2S4 nanocrystals on AgVO3 nanorod surfaces. The optimized AgVO3/CaIn2S4 heterostructure demonstrates an enhanced photocatalytic efficiency (94.1%) toward tetracycline hydrochloride (TCH) degradation compared with bare AgVO3 (42.6%) and CaIn2S4 (81.6%). The significant enhancement of photocatalytic activity is attributed to the S-scheme charge transfer mechanism in the AgVO3/CaIn2S4 heterostructure, which effectively directs photogenerated charge migration, boosts charge transfer, and preserves the high redox capacity of photoexcited electrons and holes on different active sites. This study is expected to offer insights into strategically designing and preparing S-scheme heterojunction photocatalysts to improve water purification.
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