Abstract

The design of complex, competing effects in magnetic systems—be it via the introduction of nonlinear interactions1–4, or the patterning of three-dimensional geometries5,6—is an emerging route to achieve new functionalities. In particular, through the design of three-dimensional geometries and curvature, intrastructure properties such as anisotropy and chirality, both geometry-induced and intrinsic, can be directly controlled, leading to a host of new physics and functionalities, such as three-dimensional chiral spin states7, ultrafast chiral domain wall dynamics8–10 and spin textures with new spin topologies7,11. Here, we advance beyond the control of intrastructure properties in three dimensions and tailor the magnetostatic coupling of neighbouring magnetic structures, an interstructure property that allows us to generate complex textures in the magnetic stray field. For this, we harness direct write nanofabrication techniques, creating intertwined nanomagnetic cobalt double helices, where curvature, torsion, chirality and magnetic coupling are jointly exploited. By reconstructing the three-dimensional vectorial magnetic state of the double helices with soft-X-ray magnetic laminography12,13, we identify the presence of a regular array of highly coupled locked domain wall pairs in neighbouring helices. Micromagnetic simulations reveal that the magnetization configuration leads to the formation of an array of complex textures in the magnetic induction, consisting of vortices in the magnetization and antivortices in free space, which together form an effective B field cross-tie wall14. The design and creation of complex three-dimensional magnetic field nanotextures opens new possibilities for smart materials15, unconventional computing2,16, particle trapping17,18 and magnetic imaging19.

Highlights

  • We consider a model system that consists of two intertwined, yet spatially separated, ferromagnetic nanohelices

  • We first probe the as-grown state of the two magnetic double helices in Fig. 1f,g, where we can see that in both X-ray magnetic circular dichroism (XMCD) images the double helices are composed of a dark and a bright helix, which corresponds to the individual helices being in antiparallel-magnetized single-domain states with a quasi-tangential magnetization distribution

  • Due to the periodic geometry of the double helix, the in-plane antivortices are not isolated objects: the regular array of locked domain walls leads to an array of effective antivortices in the magnetic stray field (Fig. 4b)

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Summary

Introduction

We consider a model system that consists of two intertwined, yet spatially separated, ferromagnetic nanohelices. The XMCD projection of double helix B is different, with alternating regions of dark and bright contrast within individual helices (Fig. 1i), indicating the formation of a multidomain state with a regular array of domain walls.

Results
Conclusion

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