Abstract
In this account the authors review a novel approach to design high-performance heterogeneous acid catalysts using montmorillonites as macroligands of active metal species for various C-C bond formations and one-pot syntheses. The catalytic systems using the above heterogeneous catalysts offer significant benefits in achieving environmentally friendly organic syntheses aiming towards green and sustainable chemistry. Furthermore, the present preparation method for the immobilization of metal species within the interlayer space is strikingly simple and allows a strong protocol for creating various nanostructured and functionalized metal-cation catalysts.
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