Abstract
Water pollution, especially Pb2+, Cd2+, Co2+, and Ni2+ released from industrial and mine wastewater, harms human health and is a global environmental concern. At the same time, the effective disposal of waste concrete originating from constructs is a global challenge. In this study, carbonated recycled concrete powder (CRP) is efficiently prepared by carbonizing waste concrete powder, which not only might enhance its adsorptive performance but also sequestrate CO2 in the form of mineral carbon. Characterization techniques revealed CRP forms calcium carbonate and highly polymerized silica gel. Batch adsorption experiments indicate that the CRP is found to have strong adsorption properties. The maximum equilibrium adsorption capacities calculated by the Langmuir model were determined as 997.03, 199.56, 148.85, and 76.69 mg/g for Pb2+, Cd2+, Co2+, and Ni2+, respectively, outperforming most waste concrete and industrial wastes reported. The adsorption mechanism mainly includes electrostatic interactions, precipitation, and ion exchange. This study proposes a method to synthesize low cost, good performance, high chemical stability, and facile preparation adsorbent using waste concrete powder, with promising applications in wastewater treatment.
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