Abstract
Using the semi-empirical method presented by Stone, experimental g-factors of some oxygen-substituted aromatic radicals have been correlated with the energy-level coefficient (λ) of the odd electron Hückel molecular orbitals, and with the total spin density (Σρ0) on the oxygen atoms. Parameters obtained from plots of Δgobserved/Σρ0 against λ were used to directly estimate g-factors of the radicals studied.
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