Abstract

Compared to nature's photoelectric conversion processes, artificial devices are still far inferior in efficiency and stability. Inspired by light absorption and resonance energy transfer processes of chlorophyll, we developed a highly efficient photoelectric conversion system by introducing Carbon quantum dots (CQDs) as an electron transfer intermediary. Compared with conventional dye-sensitized semiconductor systems, the present CQD-doped system showed significantly higher photoelectric conversion efficiency, as much as 7 times that without CQDs. The CQD-doped dye/semiconductor system may provide a powerful approach to the development of highly efficient photoelectric devices.

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