Abstract

Abstract. Urban areas, which are home to the majority of today's world population, are responsible for more than two-thirds of the global energy-related carbon dioxide emissions. Given the ongoing demographic growth and rising energy consumption in metropolitan regions particularly in the developing world, urban-based emissions are expected to further increase in the future. As a consequence, monitoring and independent verification of reported anthropogenic emissions is becoming more and more important. It is demonstrated using SCIAMACHY nadir measurements that anthropogenic CO2 emissions can be detected from space and that emission trends might be tracked using satellite observations. This is promising with regard to future satellite missions with high spatial resolution and wide swath imaging capability aiming at constraining anthropogenic emissions down to the point-source scale. By subtracting retrieved background values from those retrieved over urban areas we find significant CO2 enhancements for several anthropogenic source regions, namely 1.3 ± 0.7 ppm for the Rhine-Ruhr metropolitan region and the Benelux, 1.1 ± 0.5 ppm for the East Coast of the United States, and 2.4 ± 0.9 ppm for the Yangtze River Delta. The order of magnitude of the enhancements is in agreement with what is expected for anthropogenic CO2 signals. The larger standard deviation of the retrieved Yangtze River Delta enhancement is due to a distinct positive trend of 0.3 ± 0.2 ppm yr−1, which is quantitatively consistent with anthropogenic emissions from the Emission Database for Global Atmospheric Research (EDGAR) in terms of percentual increase per year. Potential contributions to the retrieved CO2 enhancement by several error sources, e.g. aerosols, albedo, and residual biospheric signals due to heterogeneous seasonal sampling, are discussed and can be ruled out to a large extent.

Highlights

  • Methods and sions is becoming more and more important

  • To determine if regionally elevated CO2 originating from anthropogenic emissions can be detected, we selected the three important CO2 source regions shown in Fig. 2 exhibiting the largest emissions in their respective continents: the RhineRuhr metropolitan region and the Benelux in Central Europe, the East Coast of the United States, and the Yangtze

  • As aerosols and albedo potentially differ between urban and background regions, Figs. 3 and 4 show aerosol optical depth (AOD) reanalysis data generated within the European GEMS (Global and regional Earth-system Monitoring using Satellite and in-situ data) project (Morcrette et al, 2009; Benedetti et al, 2009), which have been sampled at the time and location of the SCIAMACHY measurements, as well as retrieved albedo at 760 nm and 1570 nm (O2 and CO2 fitting window) www.atmos-chem-phys.net/13/2445/2013/

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Summary

Introduction

The most important anthrDopaotgaenSicygsreteenmhosuse gas carbon ments that anthropogenic CO2 emissions can be detected dioxide (CO2), which contributes substantially to global clifrom space and that emission trends might be tracked us- mate change, has increased significantly since pre-industrial ing satellite observations. This is promising with regard to future satellite missions with high spatial resolution and wide swath imaging capability aiming at constraining anthrotimes with atmospheric aGbunedoanscce ineonwtibfeicing about 40 %. Current emission invenlarger standard deviation of the retrieved Yangtze River Delta enhancement is due to a distinct positive trend of 0.3 ±

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