Abstract
The purely organic paramagnetic charge-transfer salt (TTF)3(PO-CON(CH3)C2H4SO3)2 was prepared. The anisotropic anion forms a head-to-head arrangement in the anionic layer, giving dual donor layers with different oxidation states. SQUID magnetometry indicates that spins are localized not only on the free radical (PO) but also on both TTF layers.
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