Abstract
The preparation of charge-transfer (CT) salts of DODHT [(L4-dioxane-2,3-diyldithio) dihydrotetrathia-fulvalene], BDH-TTP [2,5-bis(1,3-dithiolan-2-ylidene)-1,3,4,6-tetrathiapentalene] and BDA-TTP [2,5-bis(1,3-dithian-2-ylidene)-1,3,4,6-tetrathiapentalene] has been investigated to develop new organic superconductors. The DODHT and BDA-TTP donors give organic superconductors (DODHT) 2 BF 4 .H 2 O and (BDA-TTP) 2 X (X = GaCl 4 and FeCl 4 ) under applied pressures, whereas (BDH-TTP)Br 0.88 and (BDA-TTF) 2 X (X = BF 4 , BF 4 .H 2 O and ClO 4 ) fail to exhibit superconductivity at ambient pressure.
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