Abstract
The authors describe a laboratory computer-controlled CARS spectrometer with a single-longitudinal-mode Nd:YAG laser as a basic pump source in combination with narrowband and broadband dye lasers as Stokes sources. The frequency-stabilized pulsed Nd:YAG laser and an ultrabroadband dye laser ensure reproducible single-shot CARS spectra making the system suitable for rapid laser diagnostics.
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