Abstract

This study reports a multi-year (2000–2009) aerosol characterization for metropolitan Tehran and surrounding areas using multiple datasets (Moderate Resolution Imaging Spectroradiometer (MODIS), Multi-angle Imaging Spectroradiometer (MISR), Total Ozone Mapping Spectrometer (TOMS), Goddard Ozone Chemistry Aerosol Radiation and Transport (GOCART), and surface and upper air data from local stations). Monthly trends in aerosol characteristics are examined in the context of the local meteorology, regional and local emission sources, and air mass back-trajectory data. Dust strongly affects the region during the late spring and summer months (May–August) when aerosol optical depth (AOD) is at its peak and precipitation accumulation is at a minimum. In addition, the peak AOD that occurs in July is further enhanced by a substantial number of seasonal wildfires in upwind regions. Conversely, AOD is at a minimum during winter; however, reduced mixing heights and a stagnant lower atmosphere trap local aerosol emissions near the surface and lead to significant reductions in visibility within Tehran. The unique meteorology and topographic setting makes wintertime visibility and surface aerosol concentrations particularly sensitive to local anthropogenic sources and is evident in the noteworthy improvement in visibility observed on weekends. Scavenging of aerosol due to precipitation is evident during the winter when aconsistent increase in surface visibility and concurrent decrease in AOD is observed in the days after rain compared with the days immediately before rain.

Highlights

  • Aerosol particles impact the planet’s energy balance, the hydrological cycle, atmospheric visibility, and public health

  • Modern-Era Retrospective Analysis for Research and Applications (MERRA) are used in conjunction with the radiosonde soundings to determine the monthly trends in mixing layer heights, which have important consequences for the seasonal changes in the vertical transport and mixing of aerosols

  • To understand the importance of this interaction for the climatology of Tehran, we investigate the difference in aerosol immediately before and after rainy days, which are defined as days with observed rainfall at Mehrabad

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Summary

Introduction

Aerosol particles impact the planet’s energy balance, the hydrological cycle, atmospheric visibility, and public health. Particulate matter has been extensively monitored in several major urban centers of the world such as Beijing, Mexico City, and Los Angeles, but one area that has received disproportionately less attention in terms of examining the nature and character of aerosol is in the arid Middle East. This area is of importance with regard to air pollution owing to the large population, unfavorable topography for ventilation, and substantial sources of natural and anthropogenic emissions. It was reported that in the city of Zanjan, just to the northeast of Tehran, the dominant aerosol type was dust and that only 20% of all particles were smaller than 1 μm [12]

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