Abstract
Singles networks: The use of 1,3-propanediol and of 2-methyl-1,3-propanediol in manganese carboxylate chemistry leads to two new 3D coordination polymers with an unprecedented Mn19 repeating unit. The polymers have open framework structures with nanometer-sized cavities (see picture; Na not visible, Mn blue, O red, C gray). The Mn19 units have a ground spin state of S=23/2 and behave as single-molecule magnets.
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